Two-dimensional Pt@g-C3N4/ReS2 Van Der Waals Heterostructure for photocatalytic hydrogen evolution with direct<i> Z</i>-scheme

doi:10.1016/j.cplett.2025.142101

	Two-dimensional Pt@g-C3N4/ReS2 Van Der Waals Heterostructure for photocatalytic hydrogen evolution with direct Z-scheme
	Wang, Hong-Yao 1; Yang, Chuan-Lu 1,2; Li, Xiaohu2,3,4 ; Liu, Yuliang 1; Zhao, Wenkai 1; Gao, Feng 5
	2025-07-01
Source Publication	CHEMICAL PHYSICS LETTERS
ISSN	0009-2614
Volume	870 Pages:142101
Contribution Rank	3
Abstract	To overcome the limitations of the Pt@g-C3N4 monolayer in driving the oxygen evolution reaction (OER), we construct a photocatalytic Z-scheme with Pt@g-C3N4/ReS2 heterojunction. Band edge arrangement satisfies the requirements for hydrogen evolution reaction (HER) and OER, with a solar-to-hydrogen efficiency of 15.31 %. Nonadiabatic molecular dynamics simulation indicates that the reduction and oxidation activities of OER and HER can be efficiently protected. The Gibbs free energies indicate that the heterostructure can spontaneously drive HER, while OER requires a cocatalyst or sacrificial agent. These findings demonstrate the potential of Pt@g-C3N4/ReS2 heterojunctions as promising candidates for photocatalytic water splitting applications.
Keyword	Heterostructure Photocatalytic Direct Z -scheme Solar-to-hydrogen Gibbs free energy
DOI	10.1016/j.cplett.2025.142101
Indexed By	SCI
Language	英语
WOS Keyword	TOTAL-ENERGY CALCULATIONS ; VISIBLE-LIGHT ; CHARGE SEPARATION ; EFFICIENT ; HETEROJUNCTION ; DYNAMICS ; G-C3N4
Funding Project	National Natural Science Foundation of China[12374232] ; National Natural Science Foundation of China[12473025]
WOS Research Area	Chemistry ; Physics
WOS Subject	Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS ID	WOS:001476200700001
Publisher	ELSEVIER
Funding Organization	National Natural Science Foundation of China
Citation statistics	Cited Times:1[WOS] [WOS Record] [Related Records in WOS]
Document Type	期刊论文
Identifier	http://ir.xao.ac.cn/handle/45760611-7/7722
Collection	射电天文研究室_天体化学研究团组
Corresponding Author	Yang, Chuan-Lu
Affiliation	1.Ludong Univ, Sch Phys & Optoelect Engn, Yantai 264025, Peoples R China 2.Chinese Acad Sci, Xinjiang Astron Observ, Urumqi 830011, Peoples R China 3.Xinjiang Key Lab Radio Astrophys, Urumqi 830011, Xinjiang, Peoples R China 4.Chinese Acad Sci, Key Lab Radio Astron & Technol, Beijing 100101, Peoples R China 5.Southern Univ & A&M Coll, Dept Phys, Baton Rouge, LA 70813 USA
Corresponding Author Affilication	Xinjiang Astronomical Observatory, Chinese Academy of Sciences
Recommended Citation GB/T 7714	Wang, Hong-Yao,Yang, Chuan-Lu,Li, Xiaohu,et al. Two-dimensional Pt@g-C3N4/ReS2 Van Der Waals Heterostructure for photocatalytic hydrogen evolution with direct Z-scheme[J]. CHEMICAL PHYSICS LETTERS,2025,870:142101.
APA	Wang, Hong-Yao,Yang, Chuan-Lu,Li, Xiaohu,Liu, Yuliang,Zhao, Wenkai,&Gao, Feng.(2025).Two-dimensional Pt@g-C3N4/ReS2 Van Der Waals Heterostructure for photocatalytic hydrogen evolution with direct Z-scheme.CHEMICAL PHYSICS LETTERS,870,142101.
MLA	Wang, Hong-Yao,et al."Two-dimensional Pt@g-C3N4/ReS2 Van Der Waals Heterostructure for photocatalytic hydrogen evolution with direct Z-scheme".CHEMICAL PHYSICS LETTERS 870(2025):142101.

Files in This Item:
File Name/Size	DocType	Version	Access	License
Wang-2025-Two-dimens（4599KB）	期刊论文	出版稿	开放获取	CC BY-NC-SA	View Application Full Text

File name:	Wang-2025-Two-dimensional Pt@g-C3N4_ReS2 Van D.pdf
Format:	Adobe PDF

If you have any objections to this item, please fill out the form below and the administrator will contact you as soon as possible.
Content:
Email：	*
Institution:
Verification Code:	Refresh

Any comments and suggestions are welcomed.
Title:	*
Content:
Email：	*
Verification Code:	Refresh

射电天文研究室知识库